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Post: · Sorry, you’re posting your reply as a public Message, which means it can be read by everyone.Probing elementary excitation by Raman microscopy in graphene and its two-dimensional derivatives: implications for a possible magnetic phase.
We study the Raman scattering in monolayer graphene, multilayer graphene and two-dimensional (2D) graphite, where the contribution of the Raman active E-point phonons is analyzed. Our results show that, despite the similar vibrational spectra of these materials, the sharp and symmetric E » phonon of graphene is hardly excited, in contrast to the various Raman-active modes of 2D graphite that are expected to be spectrally broad. As a result, the magneto-Raman scattering displays a sharp enhancement when the magnetic field is applied perpendicular to the sample plane and the Raman modes of the different 2D materials follow the same B_{2g}-E_{g’} intensity ratio. We argue that the extraordinary coherence among the Raman modes in graphite results from the two-dimensionality and that the two-dimensionality of graphene is an essential ingredient of the observed coherence of the modes. Our theoretical analysis confirms that the magnetic phase of graphite is indeed spin polarized in the basal plane.The scarlet woman. From « The Fall of the House of Usher »
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